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@PHDTHESIS{Simons:480761,
      author       = {Simons, Thomas},
      othercontributors = {Simon, Ulrich and Palkovits, Regina},
      title        = {{I}mpedanzspektroskopie als {M}ethode zur in
                      situ-{R}eaktionsbeobachtung der {D}e{NO}x-{SCR}-{R}eaktion
                      an {Z}eolithen und verwandten {M}aterialien; 1. {A}ufl.},
      volume       = {3},
      school       = {Zugl.: Aachen, Techn. Hochsch.},
      type         = {Dissertation},
      address      = {Aachen},
      publisher    = {Apprimus-Verl.},
      reportid     = {RWTH-2015-03870},
      isbn         = {978-3-86359-338-4},
      series       = {Ergebnisse aus den Naturwissenschaften},
      pages        = {VI, 205 S. : Ill., graph. Darst.},
      year         = {2015},
      note         = {Weitere Reihen: Anorganische Chemie. - Edition Wissenschaft
                      Apprimus; Zugl.: Aachen, Techn. Hochsch., Diss., 2015},
      abstract     = {This thesis discuss in situ reaction monitoring by means of
                      impedance spectroscopy (IS). As a model reaction DeNOx-SCR
                      at zeolites was chosen. This work is based on solvate
                      supported proton transport mechanisms in zeolites. This
                      conductivity could be measured in situ using impedance
                      spectrsocopy. In a first step the descrimination of thermal
                      desorption and catalytic conversion of ammonia over pure and
                      metal-loaded zeolites was demonstrated by means of
                      temperature as well as time depending IS. For detailed
                      analysis a special-build measuring setup for simultaneous IS
                      and DRIFTS was used. Additional to zeolites a porous
                      zirconia-phosphate-based heterostructure was analyzed by
                      means of IS in this thesis. It was shown that the general
                      solvate-supported proton transport mechanisms could be
                      transfered to this new class of materials. In a third part
                      of this thesis the non-porous, semiconductiong material
                      ammonia paratungstate (APT-4) was analyzed. For this
                      material the thermal decomposition as well as the
                      transformation of tungsten suboxide to tungsten oxide was
                      monitored by in situ IS.},
      cin          = {151310 / 150000},
      ddc          = {540},
      cid          = {$I:(DE-82)151310_20140620$ / $I:(DE-82)150000_20140620$},
      typ          = {PUB:(DE-HGF)11 / PUB:(DE-HGF)3},
      urn          = {urn:nbn:de:hbz:82-rwth-2015-038703},
      url          = {https://publications.rwth-aachen.de/record/480761},
}