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@PHDTHESIS{zkaya:971512,
      author       = {Özkaya, Bünyamin},
      othercontributors = {Patureau, Frederic and Bolm, Carsten},
      title        = {{D}evelopment of copper-, silver-, and rhodium-catalyzed
                      coupling reactions},
      school       = {RWTH Aachen University},
      type         = {Dissertation},
      address      = {Aachen},
      publisher    = {RWTH Aachen University},
      reportid     = {RWTH-2023-09643},
      pages        = {1 Online-Ressource : Illustrationen, Diagramme},
      year         = {2023},
      note         = {Veröffentlicht auf dem Publikationsserver der RWTH Aachen
                      University; Dissertation, RWTH Aachen University, 2023},
      abstract     = {The first chapter of this thesis describes the attempt to
                      develop a general method for the formation of tetra-aryl
                      substituted hydrazines, which was unsuccessful and a
                      5,10-diphenyl-dihydrophenazine was formed instead under the
                      developed conditions. The generated
                      5,10-diphenyl-dihydrophenazine derivative was synthetized
                      for the very first time. The second chapter of the thesis
                      deals with the ortho-alkylation of phenols and diarylamines.
                      The method was first optimized for tert-butyl-phenol and the
                      scope was examined for phenols and some phenothiazines.The
                      catalytic system used either AgBF4 or HBF4 * Et2O.
                      Additionally, the synthetic utility was evaluated, and
                      mechanistic experiments were conducted. In the last chapter,
                      a one step synthesis for indoles starting from nitrobenzenes
                      has been developed. The reaction utilizes a two-metal
                      combination of elemental Zn as reductant and [RhCp*Cl2]2 as
                      catalyst. The scope was investigated thoroughly, and
                      mechanistic experiments were carried out. However due to the
                      complexity of the reaction, the mechanistic experiments were
                      not conclusive.},
      cin          = {152820 / 150000},
      ddc          = {540},
      cid          = {$I:(DE-82)152820_20140620$ / $I:(DE-82)150000_20140620$},
      pnm          = {2O2ACTIVATION - Development of Direct Dehydrogenative
                      Couplings mediated by Dioxygen (716136)},
      pid          = {G:(EU-Grant)716136},
      typ          = {PUB:(DE-HGF)11},
      doi          = {10.18154/RWTH-2023-09643},
      url          = {https://publications.rwth-aachen.de/record/971512},
}