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@PHDTHESIS{Kroell:974799,
      author       = {Kroell, Nils},
      othercontributors = {Greiff, Kathrin and Pomberger, Roland},
      title        = {{S}ensor-based characterization of anthropogenic material
                      systems: developing characterization methods and novel
                      applications for optimizing the mechanical recycling of
                      lightweight packaging waste},
      school       = {RWTH Aachen University},
      type         = {Dissertation},
      address      = {Aachen},
      publisher    = {RWTH Aachen University},
      reportid     = {RWTH-2023-11638},
      pages        = {1 Online-Ressource : Illustrationen, Diagramme},
      year         = {2023},
      note         = {Veröffentlicht auf dem Publikationsserver der RWTH Aachen
                      University 2024; Dissertation, RWTH Aachen University, 2023,
                      Kumulative Dissertation},
      abstract     = {Mechanical recycling of post-consumer plastic packaging is
                      characterized by a high lack of transparency due to the high
                      effort of manual material flow characterization. As a
                      consequence, optimizing collection processes in a targeted
                      manner as well as adaptively designing and operating sorting
                      and processing plants are often not possible, and confidence
                      in secondary raw materials is often missing. This
                      dissertation demonstrates how sensor technology in
                      mechanical recycling can evolve from a sorting technology
                      towards a key technology for enabling value-chain-wide
                      transparency, and what optimization potentials can be
                      derived from this enabled transparency. In the first part of
                      the dissertation, a systematic literature review was
                      conducted, which introduces a unified terminology, provides
                      a comprehensive overview of the current state of research
                      and identifies ten essential future research potentials. In
                      the second part, novel characterization methods for
                      extracting mass-based material flow compositions from
                      area/volume-based sensor data were developed. Machine
                      learning models were successfully trained to determine
                      binary compositions of plastic flakes and post-consumer
                      plastic packaging with a measurement uncertainty of 1.2
                      $vol\%$ and 2.4 $wt\%,$ respectively, across different
                      material flow presentations and compositions using
                      near-infrared (NIR) sensors. Based on the developed
                      characterization methods, two novel sensor technology
                      applications were demonstrated at industrial scale in the
                      third part. First, a sensor-based quality monitoring of
                      plastic pre-concentrates from sorting plants was developed
                      using inline NIR sensors. The results showed that for a PET
                      tray fraction as an example, sensor-based quality control of
                      mass-based product purities is possible with a measurement
                      uncertainity of 0.31 $wt\%.$ In comparison with
                      state-of-the-art sampling-based quality analyses, it was
                      shown that more than 350 kg of a 600 kg PET tray
                      pre-concentrate bale would need to be analyzed manually to
                      achieve a comparable measurement accuracy. Second, inline
                      NIR sensors were used for sensor-based process monitoring of
                      an industrial sensor-based sorting (SBS) unit. Using
                      artificial neural networks, the process data was used to
                      develop a process model that can predict the sorting
                      behavior of the SBS unit across different sorting scenarios
                      with a mean absolute error of $3.0\%.$ In summary, the
                      dissertation demonstrates the promising potentials of sensor
                      technology in optimizing the circular economy. Based on the
                      generated transparency, future process improvements can be
                      implemented in individual process stages and across value
                      chains, thus increasing the quantity and quality of recycled
                      materials and the resulting ecological and economic
                      benefits.},
      cin          = {512110 / 510000},
      ddc          = {620},
      cid          = {$I:(DE-82)512110_20140620$ / $I:(DE-82)510000_20140620$},
      typ          = {PUB:(DE-HGF)11},
      doi          = {10.18154/RWTH-2023-11638},
      url          = {https://publications.rwth-aachen.de/record/974799},
}